LAPTH-06322 CERN-TH-2022-158 KEK-TH-2454 Self-consistent extraction of spectroscopic bounds on light new physics C edric Delaunay1 2Jean-Philippe Karr3 4yTeppei Kitahara5 6 7z

2025-05-04 0 0 1.41MB 24 页 10玖币
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LAPTH-063/22, CERN-TH-2022-158, KEK-TH-2454
Self-consistent extraction of spectroscopic bounds on light new physics
C´edric Delaunay,1, 2, Jean-Philippe Karr,3, 4, Teppei Kitahara,5, 6, 7,
Jeroen C. J. Koelemeij,8, §Yotam Soreq,9, and Jure Zupan10, ∗∗
1Laboratoire d’Annecy-le-Vieux de Physique Th´eorique,
CNRS – USMB, BP 110 Annecy-le-Vieux, F-74941 Annecy, France
2Theoretical Physics Department, CERN, Esplanade des Particules 1, Geneva CH-1211, Switzerland
3Laboratoire Kastler Brossel, Sorbonne Universit´e, CNRS, ENS-Universit´e PSL,
Coll`ege de France, 4 place Jussieu, F-75005 Paris, France
4Universit´e d’Evry-Val d’Essonne, Universit´e Paris-Saclay,
Boulevard Fran¸cois Mitterrand, F-91000 Evry, France
5Institute for Advanced Research & Kobayashi-Maskawa Institute for the Origin
of Particles and the Universe, Nagoya University, Nagoya 464–8602, Japan
6KEK Theory Center, IPNS, KEK, Tsukuba 305–0801, Japan
7CAS Key Laboratory of Theoretical Physics, Institute of Theoretical Physics,
Chinese Academy of Sciences, Beijing 100190, China
8LaserLaB, Department of Physics and Astronomy, Vrije Universiteit Amsterdam,
De Boelelaan 1081, 1081 HV Amsterdam, The Netherlands
9Physics Department, Technion – Israel Institute of Technology, Haifa 3200003, Israel
10Department of Physics, University of Cincinnati, Cincinnati, Ohio 45221,USA
Fundamental physical constants are determined from a collection of precision measurements of
elementary particles, atoms and molecules. This is usually done under the assumption of the Stan-
dard Model (SM) of particle physics. Allowing for light new physics (NP) beyond the SM modifies
the extraction of fundamental physical constants. Consequently, setting NP bounds using these
data, and at the same time assuming the CODATA recommended values for the fundamental phys-
ical constants, is not reliable. As we show in this Letter, both SM and NP parameters can be
simultaneously determined in a consistent way from a global fit. For light vectors with QED-like
couplings, such as the dark photon, we provide a prescription that recovers the degeneracy with
the photon in the massless limit, and requires calculations only at leading order in the small new
physics couplings. At present, the data show tensions partially related to the proton charge radius
determination. We show that these can be alleviated by including contributions from a light scalar
with flavor non-universal couplings.
I. INTRODUCTION
Precision measurements of atomic and molecular prop-
erties play a dual role in fundamental physics. On the
one hand, assuming the Standard Model (SM) of parti-
cle physics, these are used to determine two of the SM
parameters, the fine-structure constant, α, and the elec-
tron mass, me(through the Rydberg constant R
α2mec/(2h)), along with a number of other observables
such as the charge radii and relative atomic masses of the
proton and deuteron. An example is the determination
of fundamental physical constants by the Committee on
Data of the International Science Council (CODATA) [1].
On the other hand, precision measurements can be
used to search for new physics (NP) beyond the SM. Such
searches have been conducted using measurements of sin-
gle particle observables [24], atomic systems [510], and
molecular systems [1114], see [15] for a review. The
cedric.delaunay@lapth.cnrs.fr
karr@lkb.upmc.fr
teppeik@kmi.nagoya-u.ac.jp
§j.c.j.koelemeij@vu.nl
soreqy@physics.technion.ac.il
∗∗ zupanje@ucmail.uc.edu
presence of NP would manifest itself as a discrepancy
between measurements and theoretical SM predictions.
The difficulty here is that in many cases the SM pre-
dictions depend on the fundamental physics parameters,
which in turn were extracted from data by CODATA un-
der the assumption that the SM is correct, and no NP
exists. In general, the presence of NP would affect the
extraction of fundamental constants, possibly reducing
the claimed sensitivity of NP searches. This subtlety is
more often than not ignored in the literature.
In this Letter we propose and carry out a self-
consistent determination of constraints on light NP mod-
els by performing a global fit, simultaneously extracting
the SM and NP parameters. We go well beyond the previ-
ous studies [5,6,16], which were performed only on sub-
sets of data. We pay special attention to the potentially
problematic limit of massless NP. The challenge is that
the SM predictions are calculated to a higher perturba-
tive order than the leading order (LO) NP contributions,
which can then lead to incorrect limiting behaviour for
very light NP. Below, we provide a prescription, valid to
LO in NP parameters, that corrects for such mismatches
in the theoretical predictions, and leads to the proper
massless NP limit.
The global fit shows several 3 σ(3 standard deviations)
discrepancies between observables and predictions, as-
arXiv:2210.10056v1 [hep-ph] 18 Oct 2022
2
suming the SM. These anomalies are well known: they
correspond to the measurements constituting the proton
charge radius puzzle [1719], with the addition of new
measurements of hydrogen transitions [20,21]. Refer-
ence [20] showed the tension of their 2S1/28D5/2mea-
surement with other hydrogen data is relaxed in the pres-
ence of an additional Yukawa-like interaction. Our global
analysis, which determines simultaneously both the SM
and NP parameters, shows for the first time that all these
deviations can be largely accounted for in a single NP
model – a light scalar that couples to gluons, electrons
and muons.
II. NEW PHYSICS BENCHMARK MODELS
We focus on minimal extensions of the SM, where ei-
ther a light scalar boson, φ, or a light vector boson, φµ,
is added to the spectrum of SM particles. The new light
particle is assumed to have parity conserving interactions
with the SM electrons and muons, as well as with light
quarks, resulting in couplings to neutrons and protons1.
The interaction Lagrangian is therefore given by
Lint =X
i=e,µ,n,p
giψi·φ)ψi,(1)
where Γ ·φφ, γµφµfor spin s= 0,1 bosons, respec-
tively. Taking the nonrelativistic limit for ψi, and work-
ing at LO in gi, the tree level exchange of φor φµinduces
a Yukawa-like nonrelativistic potential,
Vij
NP(r)=(1)s+1αφqiqj
emφr
r,(2)
between particles ψiand ψj, separated by a distance
r. The NP coupling constant, αφ≡ |gegp|/(4π)>0,
gives the strength of the NP induced potential between
electrons and protons. The strength of NP interactions
between fermions ψiand ψj, relative to the electron–
proton one, is given by the product of effective NP cou-
plings, qiqj, where qigi/p|gegp|. In particular, for the
electron–proton system the product of effective NP cou-
plings can take the values, qeqp=±1. For qiqj>0 the
potential (2) is attractive (repulsive) for spin 0 (1) medi-
ator φ, and vice versa for qiqj<0.
In the numerical analysis, we consider the following
benchmark NP models:
a. Dark photon. The light NP mediator is a vector
boson with couplings to the SM fermions proportional
to their electric charges. A UV complete realization is
an additional abelian gauge boson with field strength
F0
µν , that couples to the SM through the renormalizable
1Extension to parity non-conserving couplings and additional par-
ticles is straightforward.
kinetic mixing interaction, (/2)F0
µν Fµν [22], where
Fµν is the electromagnetic field strength. To LO in
this yields αφ=α2and qe=qµ=qp=1, qn= 0.
b. BLgauge boson. The difference of baryon (B)
and lepton (L) numbers is non-anomalous, and can be
gauged without introducing new fermions [23,24]. Light
BLgauge boson with gauge coupling gBLgives rise
to the NP potential in (2) with αφ=g2
BL/(4π). The
charges qe=qµ=qp=qn=1 coincide with the
dark photon ones, except for neutron. Comparison of
BLand dark photon bounds illustrates the importance
of performing spectroscopy of different isotopes of the
same species, such as hydrogen and deuterium.
c. Scalar Higgs portal. A light scalar mixing with
the Higgs boson [25,26] inherits the SM Yukawa struc-
ture, giving αφ= sin2θ meκpmp/(4πv2).1.8×1010
where v'246 GeV is the SM Higgs vacuum expectation
value, and θthe scalar mixing angle. The effective
leptonic (`=e, µ) charges are q`=m`/meκpmp,
while the effective nucleon charges (N=p, n) are
given by qN=κNmN/meκpmpwith κp'0.306(14)
and κn'0.308(14) [2732] (see also Sec. S4). Since
couplings to muons and nucleons are enhanced by
qµ/qe=mµ/me'200 and gN/qe=mN/me'2×103,
respectively, this NP benchmark highlights the relevance
of muonic atom and molecular spectroscopy.
d. Hadrophilic scalar. A scalar with q`= 0 and
qN=κNmN/meκpmp,i.e., with vanishing couplings
to leptons, highlights the importance of molecular
hydrogen ion spectroscopy as a probe of internuclear
interactions [11,14]. For expedience we take gNto
be the same as for the Higgs portal, but this could be
relaxed in general.
e. Up-lepto-darko-philic (ULD) scalar. In order to
evade strong bounds from K+π++Xinv searches,
where Xinv are invisible particles that escape the de-
tector, see Sec. V, we adopt a particular version of a
light scalar benchmark. The ULD scalar has enhanced
couplings to leptons, q`=m`/pmeκ0
pmp, and reduced
couplings to nucleons (due to couplings to only the up
quark), qN=κ0
NmN/pmeκ0
pmp, with κ0
p'0.018(5) and
κ0
n'0.016(5), and αφ=k2meκ0
pmp/(4πv2), with ka di-
mensionless parameter controlling the overall strength of
interactions, which is varied in the fit. The φis assumed
to predominantly decay to invisible states, possibly re-
lated to the dark matter, which evades constraints from
beam dump experiments. See Sec. S4 in the supplemen-
tal material for further details, including results for an
additional NP benchmark model– the scalar photon.
3
III. DATASETS
The adjustment of parameters, i.e., the fitting proce-
dure, presented in this work has been carried out using
two different datasets, CODATA18 and DATA22. The
CODATA18 dataset consists of data that was used in
the latest CODATA adjustment in Ref. [1], but restricted
only to the subset most relevant for constraining NP. This
subset contains observables related to the determination
of the Rydberg constant R, the proton and deuteron
radii, rpand rdrespectively, the fine-structure constant
α, and the relative atomic masses of the electron, pro-
ton, and deuteron: Ar(e), Ar(p) and Ar(d), respectively.
The inputs are listed in Tables S1,S3, and include theory
uncertainties in Table S2. The other observables and pa-
rameters included in the CODATA 2018 adjustment are
very weakly correlated with the selected data, and can
be neglected for our purpose.
The DATA22 dataset combines the updated CO-
DATA18 inputs with the additional data that improve
the overall sensitivity to NP (see Table S6 and S9). In
particular, we include the measurements of transition fre-
quencies in simple molecular or molecule-like systems,
the hydrogen deuteride molecular ion (HD+) [3335], and
the antiprotonic helium atom (¯p3He and ¯p4He) [36,37].
These have an enhanced sensitivity to the NP models
with mediators that have large couplings to quarks (and
thus nuclei). The three benchmark models of this type
are the Higgs portal, hadrophilic and ULD scalars, cf.
Sec II.
The CODATA18 dataset is used as a reference point
to verify the implementation of the inputs and the ad-
justment procedure, while DATA22 is used to obtain our
nominal results. The full list of data in the two datasets,
as well as further discussion of the importance of includ-
ing certain observables when constraining NP, is given in
Supplemental Material, Sections. S2 and S3.
IV. LEAST-SQUARES ADJUSTMENT WITH
NEW PHYSICS
The experimental data are compared to the theoretical
predictions with NP following the linearized least-squares
procedure [38]. The theoretical prediction for an observ-
able Otakes the form,
O=OSM(gSM) + ONP(gSM, αφ, mφ) + δOth ,(3)
where OSM is the state of the art SM predic-
tion, and depends on the SM parameters gSM =
{R, rp, rd, α, Ar(e), Ar(p), Ar(d)}, while the NP contri-
bution ONP depends in addition on αφand mφ. The
theoretical uncertainties are included as in Ref. [1], by
adding a normally distributed variable δOth with zero
mean and standard deviation equal to the estimated un-
certainty of the theoretical expression. The δOth’s are
treated as yet another set of input data and varied in the
fit, along with gSM,αφ, and mφ, in order to minimize the
χ2function constructed from the input data and theory
predictions (see also Sec. S1).
The SM theoretical predictions for atomic transi-
tion frequencies, the electron anomalous magnetic mo-
ment, and bound-electron g-factors are from Ref. [1] (see
references therein). The predictions for the HD+and
¯pHe transition frequencies are from Ref. [39,40] and [41
43], respectively, and are updated with the latest CO-
DATA recommended values, see Sec. S3 for details.
The NP contributions to atomic and molecular
ion transition frequencies are obtained using (time-
independent) first-order perturbation theory [44,45]. We
use exact nonrelativistic wavefunctions for hydrogen-like
atoms and very precise nonrelativistic numerical ones
from a variational method of Ref. [46] for HD+and ¯pHe.
Expectation values of the Yukawa potentials in Eq. (2)
are calculated for a grid of mφvalues, taking advantage
of the fact that their matrix elements in the chosen basis
can be obtained in an analytical form. The precision is
limited to O(α2) because of the neglected relativistic cor-
rections to the wavefunction. The NP contribution to the
free-electron (g2)earises at one-loop [47,48], while for
bound electrons we include an additional tree-level con-
tribution from electron-nucleus interaction [49]. Finally,
we assume NP to have negligible effects in atom recoil
measurements as well as relative atomic mass measure-
ments from cyclotron frequency measurements in Pen-
ning traps.
We pay particular attention to the possible degeneracy
between the determination of SM and NP parameters. In
the mφ0 limit, the dark photon is completely degener-
ate with the QED photon, since couplings of the two are
aligned, qi=Qi, and thus only the combination α+αφ
can be determined from data. This degeneracy should
be retained in the theoretical predictions (3), which in
principle requires calculating NP effects to the same very
high order as the SM. We propose an alternative pro-
cedure, which uses the state-of-the-art SM calculations
but requires NP contribution only at LO in αφ, and re-
produces the correct qiQi,mφa01 limit, where
a0α/(4πR)=(αme)1is the Bohr radius.
For light vectors we rewrite the NP potential in Eq. (2)
as the sum of the Coulomb-like potential with QED cou-
pling Qiplus the remainder,
Vij
NP(r) = αφ
QiQj
r+e
Vij
NP(r),(4)
where e
Vij
NP(r)αφ(qiqjemφrQiQj)/r. The theory
predictions are evaluated at LO in e
VNP(r), while the NP
Coulomb term and the related relativistic corrections are
evaluated to the same order as the SM, which amounts
to replacing αα+αφin the SM predictions. For any
observable Othe theoretical prediction is then
O=OSM (α+αφ)+ e
ONP (α+αφ, αφ, mφ),(5)
where OSM is the SM contribution now expressed as a
function of α+αφand e
ONP is the NP contribution from
4
αa0
-1
a0
-1
mμ/mea0
-
1
Higgs portal
U(1)B-L
photon
hadrophilic scalar
ULD scalar
10-410-310-210-11 10 102103104105
10-18
10-17
10-16
10-15
10-14
10-13
10-12
10-11
10-10
10-9
10-8
10-7
m
ϕ
[
keV
]
αϕ95%CL exclusion
FIG. 1. The 95% CL bounds on the NP coupling constant αφ
as a function of the new boson’s mass mφfor the benchmark
NP models of Sec. II, as indicated. Other model-dependent
constraints may apply (see text).
e
VNP. In the mφ0, qiQilimit the potential e
VNP
vanishes, and all theory predictions are the SM ones, but
shifted by αα+αφ. For massive dark photon with
mφa01 the leading effect of e
VNP is parametrically
e
ONP m2
φ. Note that for massless BLthe potential
˜
VNP vanishes in hydrogen but not in deuterium where
e
ONP qn, thus breaking the degeneracy between the
SM and NP contributions when mφ0.
For light scalars there is no degeneracy with QED in
the massless mediator limit; it is lifted by relativistic cor-
rections. We can use directly the state-of-the-art SM
predictions, and simply add to them the NP contribu-
tion due to the potential (2) at LO, without any special
treatments, see also Sec. S7.
V. RESULTS
First, we perform the control fit, i.e., the least-squares
adjustment assuming SM, based on the CODATA18
dataset with inflated experimental uncertainties when
there are tensions in the data [1], see also Sec. S2. Re-
sulting χ2per degree-of-freedom (dof) is χ2
SMdof '0.95
(νdof = 7844 = 34), indicating an overall good descrip-
tion by the SM, and the use of correct expansion fac-
tors. The output gSM values and relative uncertainties
(see Table S5) are in excellent agreement (.0.2σ) with
the latest CODATA recommended values [1], validating
our procedure.
Next, we perform adjustments based on the DATA22
dataset, assuming either the SM or one of the NP bench-
mark models in Sec. II. We do not inflate experimental
errors, since mild tensions in the data could be a hint of
NP. The SM-only hypothesis still describes the data rel-
atively well, with χ2
SMdof '1.4 (νdof = 102 62 = 40),
a0
-1
mμ/mea0
-1
NA62
SN1987a
E137
stellar
cooling
ULD scalar
1 10 102103104105
10-15
10-14
10-13
10-12
10-11
10-10
10-9
10-8
10-7
10-4
10-3
10-2
10-1
1
10
102
103
104
mϕ[keV]
αϕ
k2
FIG. 2. The constraints on ULD scalar in the αφ, mφplane,
with purple-shaded 1,2,3,4σCL regions favored by the
DATA22 dataset (black dot is the best-fit point). Exclusions
are by SN1987a [50,51] (below the pink line, absent if φin-
visible decay dominates), NA62 K+π+Xinv search [52]
(green, the dashed line is a naive NNLO estimate), stellar
cooling [53] (gray), and E137 [54,55] (between yellow dashed
lines, absent if φinvisible decay dominates).
despite known tensions in the proton charge radius puz-
zle data and the recent hydrogen 2S1/28D5/2transi-
tion [20].
Figure 1shows the 95 % confidence level (CL) up-
per bounds on αφas function of mφfor the NP bench-
mark models, Sec. II. The strongest exclusion is always
reached around mφa1
04 keV, and stays roughly
constant for lighter mφ(except for dark photon due
to degeneracy with QED in the mφ0 limit, see
Sec. IV). Deuterium observables translate to a 2×
stronger bound on BLat mφa1
0, compared to
dark photon. The significantly stronger bounds on the
Higgs portal and hadrophilic scalar for mφ.10 keV are
due to the κpmp/me'500 enhancement in inter-
nucleon interactions (compared to electron–nucleon po-
tential), affecting the HD+observables. For heavier NP,
mφa0&1 (mµ/me) in hydrogen (muonic hydrogen),
the interaction is point-like, with suppressed electron
(muon) wave function overlap, and the bounds decou-
ple as 1/m2
φ(and more quickly for hadrophilic scalar).
The bounds are stronger for Higgs portal and ULD scalar
due to mµ/me'200 enhanced effects in muonic hy-
drogen.
For mφa0&mµ/methe Higgs portal and ULD scalar
are statistically preferred over the SM at the 4σand
5σlevel, respectively. Figure 2shows the preferred
region for the ULD scalar, around the best-fit point,
mφ= 300 keV and αφ= 6.7×1011. This NP hint
is supported mostly from the recent measurements of
the hydrogen 2S1/28D5/2and 1S1/23S1/2transi-
tions [20,21], as well as muonic deuterium, cf. Sec. S5.
While these tensions between data and the SM predic-
5
Higgs portal
mϕ=400keV
ULD scalar
mϕ=300keV
SM
DATA22
CODATA18
CODATA18 (no expansion factors)
0 5 10 15 20
-2
0
2
4
6
(rp-rp
2018)/u(rp
2018)
(R-R
2018)/u(R
2018)
FIG. 3. The 68% CL regions for simultaneous determina-
tions of the Rydberg constant Rand the proton radius rp
assuming either the SM-only hypothesis (gray) or including
putative NP contributions from a 400 keV Higgs portal scalar
(blue) or 300 keV ULD scalar (purple). The solid lines use
DATA22 dataset, the dashed (dotted) lines the CODATA18
dataset with (without) errors inflated by expansion factors.
Both Rand rpare shown in terms of normalized devia-
tions from the central values of the CODATA 2018 analysis,
Ref. [1].
tion are not new, our analysis shows that all tensions
can be significantly ameliorated when including NP in-
teractions due to a single light scalar. The favored NP
mass is close to the (inverse) Bohr radius of muonic
atoms, a1
0×mµ/meMeV, due to the large muon-
electron coupling ratio in these models, contrasting with
scalars having weaker or vanishing coupling to muons (see
Sec. S4 and [20]). However, other constraints require the
scalar to have rather a nontrivial pattern of couplings, see
Sec S4 A. For ULD scalar the E137 [54,55] bounds are
evaded since φdecays predominantly to an invisible dark
sector. Since φcouples to up quarks and not directly to
heavy quarks and gluons, the bound from NA62 search
for K+π+φ[52] is weakened [51,56]. Finally, the
minimal ULD model induces a too large contribution to
(g2)µ, however this can be suppressed in less minimal
versions with a custodial symmetry [57].
The presence of NP also impacts the determination
of the fundamental constants in the SM. Figure 3
shows the 68 % CL determination of rpand R, sub-
tracting the CODATA 2018 recommended values and
normalizing to respective errors. The SM-parameter
uncertainties increase in the presence of NP and the
central values shift outside the nominal SM ellipse,
shown explicitly in Fig. 3for the Higgs portal and
ULD scalar model. Because of the degeneracy with
the photon the uncertainty on αin the dark photon
model increases as 1/m2
φfor masses below 10 eV (see
Fig. S7) and eventually becomes comparable to αitself
for mφ0.1 meV, while α+αφremains well constrained.
VI. CONCLUSIONS
Extracting bounds on light NP from a global fit to
spectroscopic and other precision data requires both SM
and NP parameters to be determined simultaneously.
The possibility of NP contributions changes the extracted
allowed ranges of SM parameters, a change that can be
quite substantial, see Fig. 3. Furthermore, we provided a
prescription to consistently include NP corrections from
light vectors. It requires calculations of NP contribution
only at leading order, and recovers the expected degener-
acy between dark photon and QED in the massless me-
diator limit.
At present, spectroscopic data show tensions that
could either be due to unknown or under-appreciated
systematics, or to light NP. We showed that the 4σ
anomaly in data can be explained by a flavor non-
universal light scalar model.
ACKNOWLEDGMENTS
We would like to thank Dmitry Budker and Gi-
lad Perez for useful discussions and comments on the
manuscript. The work of CD is supported by the
CNRS IRP NewSpec. The work of TK is supported
by the Japan Society for the Promotion of Science
(JSPS) Grant-in-Aid for Early-Career Scientists (Grant
No. 19K14706) and the JSPS Core-to-Core Program
(Grant No. JPJSCCA20200002). The work of YS is sup-
ported by grants from the NSF-BSF (No. 2018683),
the ISF (No. 482/20), the BSF (No. 2020300) and
by the Azrieli foundation. JZ acknowledges support in
part by the DOE grant de-sc0011784. This work was
also supported in part by the European Union’s Hori-
zon 2020 research and innovation programme, project
STRONG2020, under grant agreement No. 824093.
[1] E. Tiesinga, P. J. Mohr, D. B. Newell, and
B. N. Taylor, “CODATA recommended values of the
fundamental physical constants: 2018*,” Rev. Mod.
Phys. 93 (2021) 025010.
[2] D. Hanneke, S. Fogwell, and G. Gabrielse, “New
Measurement of the Electron Magnetic Moment and
the Fine Structure Constant,” Phys. Rev. Lett. 100
(2008) 120801 [arXiv:0801.1134].
摘要:

LAPTH-063/22,CERN-TH-2022-158,KEK-TH-2454Self-consistentextractionofspectroscopicboundsonlightnewphysicsCedricDelaunay,1,2,Jean-PhilippeKarr,3,4,yTeppeiKitahara,5,6,7,zJeroenC.J.Koelemeij,8,xYotamSoreq,9,{andJureZupan10,1Laboratoired'Annecy-le-VieuxdePhysiqueTheorique,CNRS{USMB,BP110Annecy-le-V...

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