Droplet Arrays in Doubly-Dipolar Bose-Einstein condensates Ratheejit Ghosh1Chinmayee Mishra1 2Luis Santos3and Rejish Nath1 1Department of Physics Indian Institute of Science Education and Research Pune Pune 411 008 India

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Droplet Arrays in Doubly-Dipolar Bose-Einstein condensates
Ratheejit Ghosh,1Chinmayee Mishra,1, 2 Luis Santos,3and Rejish Nath1
1Department of Physics, Indian Institute of Science Education and Research Pune, Pune 411 008, India
2Indian Institute of Technology Gandhinagar, Gandhinagar 382 355, India
3Institut f¨ur Theoretische Physik, Leibniz Universit¨at Hannover, Appelstrasse 2, DE-30167 Hannover, Germany
(Dated: October 28, 2022)
Gases of doubly-dipolar particles, with both magnetic and electric dipole moments, oer intriguing novel pos-
sibilities. We show that the interplay between doubly-dipolar interactions, quantum stabilization, and external
confinement results in a rich ground-state physics of supersolids and incoherent droplet arrays in doubly-dipolar
condensates. Our study reveals novel possibilities for engineering quantum droplets and droplet supersolids,
including supersolid-supersolid transitions and the realization of supersolid arrays of pancake droplets.
I. INTRODUCTION
The anisotropic and long-range nature of the dipole-dipole
interactions leads to a rich physics in dipolar quantum gases,
qualitatively dierent than that of their non-dipolar counter-
parts [13], including anisotropic superfluidity [46], roton-
like excitations [7,8], and the recent realization of quantum
droplets [912]. The latter result from the interplay between
contact and dipolar interactions and the stabilization provided
by quantum fluctuations [13]. Interestingly, the external con-
finement may result in the formation of arrays of droplets,
which under proper conditions may remain mutually coher-
ent, building a dipolar supersolid [1417], whose properties
have recently been the focus of major attention [1726].
Experiments on dipolar Bose-Einstein condensates have
been realized so far with atoms with large permanent magnetic
moments such as chromium [27,28], erbium [29], and dys-
prosium (Dy) [30]. Interestingly, a pair of quasi-degenerate
states with opposite parity oers the possibility of inducing an
additional electric dipole moment in Dy atoms using an elec-
tric field [31]. Recently, doubly-dipolar atoms and molecules
possessing both electric and magnetic dipole moments [31
39] have attracted a large deal of interest due to their poten-
tial applications in quantum simulation [40], computing [41],
tests of fundamental symmetries [42], and for the tuning of
collisions and chemical reactions [43]. Interestingly, the elec-
tric and magnetic moments may be oriented in dierent di-
rections, opening novel possibilities for doubly-dipolar con-
densates [44]. Self-bound quantum droplets may undergo a
dimensional crossover when varying the angle between the
dipole moments without modifying the external confinement.
In this paper, we show that the control of the relative angle
between the two dipole moments opens new intriguing sce-
narios for quantum droplet arrays in doubly-dipolar conden-
sates, including a density-modulated single droplet ground-
state, supersolid-supersolid transitions, and the possibility of
realizing an array of pancake-shaped quantum droplets.
The paper is structured as follows. In Sec. II, we re-
view a particular realization of a doubly-dipolar system us-
ing dysprosium atoms, employed in the rest of the paper. In
Sec. III, we discuss the anisotropic properties of the dou-
bly dipolar potential. In Sec. IV, we introduce the extended
Gross-Pitaevskii equation for a doubly-dipolar condensate, in-
corporating beyond-mean-field corrections. The properties of
a single self-bound droplet are briefly discussed in Sec. V.
Section VI is devoted to analyzing quantum droplet arrays in
doubly-dipolar condensates. Finally, we summarize our con-
clusions in Sec. VII.
II. DOUBLY-DIPOLAR DYSPROSIUM ATOMS
In this section, we discuss a particular realization of a
doubly-dipolar system using Dy atoms, briefly reviewing the
proposal of Ref. [31]. However, other realizations, e.g. using
molecules, should result in a similar physics.
In addition to its permanent magnetic moment, an electric
moment may be induced in Dy atoms by an external electric
field owing to a pair of quasi-degenerate states with oppo-
site parity. These states, |ai(odd parity) and |bi(even par-
ity), have total angular momenta {Ja=10,Jb=9}, and en-
ergies {Ea=17513.33 cm1,Eb=17514.50 cm1}. Within
the electric-dipole approximation, the line-widths of the states
are Γa0 (metastable) and Γb=2.98 ×104s1, respec-
tively. We assume that the Dy atoms are in uniform mag-
netic and electric fields. The magnetic field, B=Bˆz, is
directed along z, setting the quantization axis and splitting
the degeneracy of the energy levels Eaand Eb. The elec-
tric field, E=Eˆumixes the Zeeman sublevels of the states,
{|Ma=Jai, ..., |+Jai,|Mb=Jbi, ..., |+Jbi}, inducing an
electric dipole moment along ˆu. We assume that ˆulies on
the xz plane forming an angle αwith the z-axis. This relative
angle plays a crucial role in the physics discussed below.
Restricting to the subspace of both Eaand Eb, the Hamilto-
nian for a Dy atom is ˆ
H=ˆ
HB+ˆ
Hstark with
ˆ
HB=EaX
Ma|MaihMa|+EbX
Mb|MbihMb|+µBB(gaMa+gbMb),
(1)
where ga=1.3 and gb=1.32 are the Land´
egfactors. The
term ˆ
Hstark accounts for the interaction of the electric field
with the Dy atom. The electric field strength is such that the
lowest eigenstate of the atom is |Si=c0|Ma=10i+P0
ici|ii
with P0
i|ci|2/|c0|21, where the sum P0
iis taken over all the
magnetic sublevels except |Ma=10i, and ciis the probabil-
ity amplitude for finding the atom in the state |ii. The summa-
tion P0
ihas two contributions, one from the sublevels of |ai
and the other from those of |bi. Since Γa0, only the con-
tributions from the sublevels {|Mbi} determine the lifetime of
arXiv:2210.01093v2 [cond-mat.quant-gas] 27 Oct 2022
2
0
0
0.5
0.1 0.2 0.3 0.4
0
00.40.30.2 0.5
0.1
Figure 1. (Color online) (a) Electric dipole moment deand (b) life-
time τof the |Sistate of a Dy atom, as a function of the electric field
strength Eand the angle αbetween the electric and magnetic fields
for B=100 G.
the stretched state |Si,τ=(nbΓb)1, where nbis the total pop-
ulation in {|Mbi} sublevels. The magnetic and electric dipole
moments of a Dy atom in |Siare, respectively:
dm=µB
ga
Ja
X
Ma=Ja|cMa|2Ma+gb
Jb
X
Mb=Jb|cMb|2Mb
(2)
de=1
EX
Ma,Mb
c
MacMbhMa|ˆ
Hstark|Mbi+c.c.(3)
with
hMa|ˆ
Hstark|Mbi=s4π
3(2Ja+1) ha|| ˆ
d||biE ×
Y
1,MaMb(α, 0) CJaMa
JbMb,1,MaMb,(4)
where, ha|| ˆ
d||bi=8.16 Debye is the reduced transition
dipole moment, Yl,m(θ, φ) are the spherical harmonics and
CJaMa
JbMb,1,MaMbare the Clebsch-Gordan coecients.
Figure 1depicts, for B=100 G, deand dmfor the state
|Si, as a function of Eand α. When α=0, the spherical
harmonics, Y
1,MaMb(α, 0) are non-zero only when Ma=Mb
and thus, the electric field couples pairs of sublevels with
Ma=Mb. Since the state |Ma=10ihas no counterpart
in the {|Mbi} subspace, the former is unaected by the electric
field. Hence, the electric dipole moment of the Dy atom in
the state |Sivanishes for α=0. When αgrows, the electric
field couples |Ma=10iwith other |Mbisublevels, reach-
ing a maximum mixing for α=π/2 (see Fig. 1(a)). There-
fore, for a given E,deincreases with αuntil α=π/2. This
comes at the cost of decreasing the lifetime of |Si, as shown
in Fig. 1(b). For a range of experimentally realistic E=0-4
Figure 2. (Color online) Doubly-dipolar atoms. Both electric (de)
and magnetic (dm) dipoles are assumed polarized on the xz plane,
forming an angle αbetween them. The angle θm(θe) is the angle
between dm(de) and the vector joining the atoms, r.
kV/cm, devaries from 0 to 0.16 Debye and the magnetic mo-
ment remains constant, dm'13 µB(higher than ground-state
Dy atoms), whereas the lifetime of |Sivaries from 28 s (con-
sidering electric-quadrupole and magnetic-dipole transitions)
to 10 ms [31].
III. DOUBLY DIPOLAR POTENTIAL
The doubly-dipolar interaction between two atoms is
Vd(r)=µ0d2
m
4π
(1 3 cos2θm)
|r|3+d2
e
4π0
(1 3 cos2θe)
|r|3(5)
where µ0(0) is the vacuum permeability (permittivity) and
θm(θe) is the angle formed by the magnetic (electric) dipole
moment with the vector rjoining the atoms (Fig. 2). Whereas
Vd(r) is always repulsive along the y-axis, it is anisotropic
on the xz-plane. This anisotropy is well characterized by the
angular part of the dipolar potential on the xz-plane:
Vy=0
d(r, θ)"13cos2θ+γ(cos θcos α+sin αsin θ)2
1+γ#,(6)
where θis the polar angle, and γ=(de/dm)2/(µ00) char-
acterizes the relative strength between the electric and mag-
netic dipole moments. The ratio γcan be varied indepen-
dently of αby tuning E. In Fig. 3, we depict Vy=0
d(r) for
dierent αand γ. When α=0, we have the usual dipolar
potential, attractive along zand repulsive along x[3]. As
αincreases up to π/2, the dependence of the potential on
γbecomes more significant. For α=π/2, when γgrows
the potential inverts eventually its anisotropy (last column of
Fig. 3). If 4γ2+γ49γ, there exists a critical angle
1
2cos1h(4γ2+γ4)/9γiabove which the xz potential be-
comes purely attractive (see Figs. 3(g), (h), and (l)), but re-
mains anisotropic except when α=π/2 and γ=1. For that
case Vy=0
d(r, θ)=1/r3.
Despite this nontrivial anisotropy, we may define an eec-
tive polarization axis, depicted by arrows in Fig. 3, given by
摘要:

DropletArraysinDoubly-DipolarBose-EinsteincondensatesRatheejitGhosh,1ChinmayeeMishra,1,2LuisSantos,3andRejishNath11DepartmentofPhysics,IndianInstituteofScienceEducationandResearchPune,Pune411008,India2IndianInstituteofTechnologyGandhinagar,Gandhinagar382355,India3Institutf¨urTheoretischePhysik,Leibn...

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Droplet Arrays in Doubly-Dipolar Bose-Einstein condensates Ratheejit Ghosh1Chinmayee Mishra1 2Luis Santos3and Rejish Nath1 1Department of Physics Indian Institute of Science Education and Research Pune Pune 411 008 India.pdf

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