Colloquium Spin-orbit effects in superconducting hybrid structures Morten Amundsen Nordita KTH Royal Institute of Technology and Stockholm University

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Colloquium: Spin-orbit effects in superconducting hybrid structures
Morten Amundsen
Nordita, KTH Royal Institute of Technology and Stockholm University,
Hannes Alfvéns väg 12, SE-106 91 Stockholm, Sweden
Center for Quantum Spintronics, Department of Physics, Norwegian University of Science & Technology,
NO-7491 Trondheim, Norway
Jacob Linder
Center for Quantum Spintronics, Department of Physics, Norwegian University of Science & Technology,
NO-7491 Trondheim, Norway
Jason W. A. Robinson
Department of Materials Science & Metallurgy, University of Cambridge, 27 Charles Babbage Road,
Cambridge CB3 0FS, United Kingdom
Igor Žutić
Department of Physics, University at Buffalo, State University of New York, Buffalo, New York 14260, USA§
Niladri Banerjee
Department of Physics, Blackett Laboratory, Imperial College London, London SW7 2AZ, United Kingdom
Spin-orbit coupling (SOC) relates to the interaction between an electron’s motion and its spin, and is
ubiquitous in solid-state systems. Although the effect of SOC in normal-state phenomena has been
extensively studied, its role in superconducting hybrid structures and devices opens many unexplored
questions. In conjunction with broken symmetries and material inhomogeneities within supercon-
ducting hybrid structures, SOC may have additional contributions, beyond its effects in homogenous
materials. Remarkably, even with well-established magnetic or nonmagnetic materials and conven-
tional s-wave spin-singlet superconductors, SOC leads to emergent phenomena including equal-spin
triplet pairing and topological superconductivity (hosting Majorana states), a modified current-phase
relationship in Josephson junctions, and nonreciprocal transport. SOC is also responsible for trans-
forming quasiparticles in superconducting structures which enhances the spin Hall effect and changes
spin dynamics. Taken together, SOC in superconducting hybrid structures and the potential for elec-
tric tuning of the SOC strength, creates fascinating possibilities to advance superconducting spintronic
devices for energy-efficient computing, and enable topological fault-tolerant quantum computing. By
providing a description of experimental techniques and theoretical methods to study SOC, this Collo-
quium describes the current understanding of resulting phenomena in superconducting structures and
offers a framework to select and design a growing class of materials systems where SOC plays an
important role.
CONTENTS
I. Introduction 2
II. Background 3
A. Spin–orbit coupling 3
B. Validity of Rashba and Dresselhaus models 4
C. Triplet superconductivity 5
D. Theoretical frameworks 6
1. General considerations of spin-dependent fields 6
2. Superconducting proximity effect 7
3. The Ginzburg-Landau formalism 8
4. Bogoliubov-de Gennes method 9
5. Quasiclassical theory 9
Corresponding author:morten.amundsen@ntnu.no
Corresponding author:jacob.linder@ntnu.no
Corresponding author:jjr33@cam.ac.uk
§Corresponding author:zigor@buffalo.edu
Corresponding author:n.banerjee@imperial.ac.uk
III. Experimental techniques 11
A. Transition temperature measurements 11
B. Josephson junctions 11
C. Magnetization dynamics 11
D. Spectroscopic techniques 12
E. Low-energy muon spin rotation technique 12
IV. Recent developments 12
A. Majorana zero modes 13
B. Superconducting critical temperature 15
C. Modification of magnetic anisotropy 15
D. Interfacial magnetoanisotropy 16
E. Josephson junctions 17
F. Supercurrent diodes 20
G. Spin-pumping 21
H. Spin-Hall phenomena with superconductors 21
V. Open questions and future directions 23
Acknowledgments 24
References 26
arXiv:2210.03549v2 [cond-mat.supr-con] 1 Jul 2024
2
I. INTRODUCTION
As a relativistic effect, the motion of an electron in an elec-
tric field creates a magnetic field in its rest frame (Jackson,
1998). The resulting spin-orbit coupling (SOC) in solid-state
systems can have different contributions. In addition to the
coupling of electron spin with the average electric field from
the periodic crystal potential, other SOC terms arise due to
an applied or built-in electric field, for example due to broken
inversion symmetry. One can also distinguish intrinsic, ex-
trinsic, and synthetic SOC, due to electronic structure, impuri-
ties, and magnetic textures, respectively. With SOC, at a given
wave vector, k, the twofold spin degeneracy is removed result-
ing in a k-dependent Zeeman energy and an effective magnetic
field (Winkler, 2003; Žuti´
cet al., 2004). In superconducting
heterostructures, the role of SOC can be even more striking
by transforming the orbital and spin symmetry of the Cooper
pairs, through which exotic states may emerge—even from
simple s-wave spin-singlet superconductors.
For decades, SOC effects have been identified as crucial
for many normal-state phenomena, such as spin-photon and
spin-charge conversion (Meier and Zakharchenya, 1984), var-
ious topological states (Armitage et al., 2018; Shen, 2012),
the family of spin Hall effects (D’yakonov and Perel’, 1971a;
Maekawa et al., 2012), magnetocrystalline anisotropy and
noncolinear spin textures (including skyrmions and chiral do-
main walls) (Tsymbal and Žuti´
c, 2019). They also formed the
basis for early spintronic applications, which can be traced
back to the discovery of anisotropic magnetoresistance in
1857 (Thomson, 1857; Žuti´
cet al., 2004). In contrast, the
relevance of SOC in superconducting structures was largely
absent, or limited to specific aspects without fully recogniz-
ing many connections (Bergeret et al., 2005; Buzdin, 2005;
Golubov et al., 2004; Meservey and Tedrow, 1994; Tedrow
and Meservey, 1971). Motivated by recent advances in stud-
ies of hybrid superconducting structures where SOC plays a
prominent role, this review aims to provide an experimental
and theoretical framework to highlight many such connec-
tions between different phenomena and emerging applications
in these structures.
The quest to realize topological superconductivity and elu-
sive Majorana states for fault-tolerant topological quantum
computing in structures with strong SOC relies on equal-spin-
triplet superconductivity (Elliot and Franz, 2015; Nayak et al.,
2008). This triplet superconductivity is also sought in super-
conducting spintronics (Eschrig, 2015; Linder and Robinson,
2015; Ohnishi et al., 2020; Yang et al., 2021) as it supports
dissipationless spin currents and allows for the coexistence of
superconductivity and ferromagnetism. Josephson junctions
(JJs) with tunable SOC, which enable spin-triplet supercon-
ductivity, are important building blocks for topological super-
conductivity and superconducting spintronics (Dartiailh et al.,
2021; Mayer et al., 2020). These JJs also reveal the supercon-
ducting diode effect (Baumgartner et al., 2022; Dartiailh et al.,
2021) an example of a nonreciprocal phenomenon (Nadeem
et al., 2023). While nonreciprocal effects are technologi-
cally important (Marder, 2010; Shockley, 1952) and known
since the nineteenth century in the normal state (Faraday,
1846; Kerr, 1877), experimental demonstrations of supercon-
ducting counterparts were largely absent, until a few years
ago (Nadeem et al., 2023). Analogous to multiferroic ma-
terials which allow electrical control of magnetic properties
and, conversely, magnetic control of electrical properties, we
can view SOC in the superconducting state as enabling vari-
ous magnetoelectric effects (Tkachov, 2017) and facilitating
the coupling between different order parameters. Since SOC
changes the properties of quasiparticles in superconductors, it
has also been shown to produce strongly enhanced spin Hall
phenomena in superconducting structures.
With controllable SOC, the previous efforts to integrate
superconductors and ferromagnets can be radically simpli-
fied. Instead of engineering complex noncollinear mag-
netic structures at the superconductor/ferromagnet (S/F) inter-
face (Banerjee et al., 2014; Keizer et al., 2006; Khaire et al.,
2010; Robinson et al., 2012, 2010; Usman et al., 2011), a sin-
gle common F with SOC in a superconducting heterostruc-
ture with broken inversion symmetry is sufficient to support
spin-triplet superconductivity and large magnetoresistive ef-
fects (Banerjee et al., 2018; Cai et al., 2021; González-Ruano
et al., 2021, 2020; Jeon et al., 2018, 2019a, 2020b; Martínez
et al., 2020). Theoretically, the observed role of SOC in
singlet-to-triplet pair conversion has been studied for both
ballistic and diffusive transport (Bergeret and Tokatly, 2013,
2014; Feng et al., 2008; Högl et al., 2015; Jacobsen et al.,
2015; Yokoyama et al., 2006) and preceded by the related
effect of spin-active interfaces (Eschrig et al., 2003; Hal-
terman and Valls, 2009; Linder et al., 2009; Žuti´
c and Das
Sarma, 1999) and SOC generated k-anisotropic triplet con-
densates (Edelstein, 2003; Gor’kov and Rashba, 2001).
Another example where SOC fundamentally modifies the
underlying physics is within superconducting random-access
memories using ferromagnetic JJs. Here, nonvolatile control
of the zero and πground state phase encoding binary informa-
tion (Birge and Houzet, 2019; Dayton et al., 2018), needs to
be revisited in the presence of SOC where, in addition to the
spin-singlet and the spin-triplet states, their admixture is also
possible. The resulting anomalous Josephson effect (Buzdin,
2008; Reynoso et al., 2008) supports an arbitrary phase shift
other than just zero and π, leading to novel challenges and
opportunities for non-binary information processing and stor-
age. Just as magnetic JJs are the building blocks for super-
conducting memories, their nonmagnetic counterparts are the
key elements for low-power and high-speed superconducting
logic (Holmes et al., 2013; Tafuri, 2019) and superconduct-
ing quantum computing (Krantz et al., 2019; Wendin, 2017).
This means that SOC may not only modify such devices, but
also provide entirely new functionalities in their operation, as
current-phase relation, Josephson energy, critical temperature
and critical current, can all strongly change with SOC. As
in the normal state, SOC is the major source of spin relax-
ation and decoherence, as well as the underlying mechanism
for spin dynamics, in the superconducting state (Žuti´
cet al.,
3
2004). Since both long and short spin relaxation times (Lin-
demann et al., 2019; Nishikawa et al., 1995) can be desirable
in the normal state, their SOC-controlled tunability in the su-
perconducting state would be similarly advantageous. Taken
together, the presence of SOC and its tunability in hybrid su-
perconducting structures offers an intriguing prospect to both
identify novel phenomena as well as advance various quantum
technologies, from storing, transferring, and processing infor-
mation, to improving quantum sensing. While some of the
resulting efforts simply extend the current concepts and appli-
cations of superconductivity, others, like topological quantum
computing, would radically change the paths towards realiz-
ing computational architectures (Cai et al., 2023). Even if the
most ambitious proposals remain aspirational, the advances in
our understanding of SOC have already transformed the way
we view various superconducting phenomena.
By focusing on more common materials, where their super-
conductivity is well established, simplifies the understanding
of the role of SOC. For example, a large part of this review
focuses on hybrids with conventional elemental or nitride s-
wave superconductors, including Nb, Al, V, and NbN. How-
ever, we note that other superconducting systems to investi-
gate SOC effects are possible; for over two decades supercon-
ducting spintronics has been studied with high-temperature d-
wave superconductors (Chen et al., 2001; Vas’ko et al., 1997;
Wei et al., 1999), where even their normal-state properties re-
main debated. In briefly mentioning other oxide supercon-
ductors, two-dimensional superconductors, such as NbSe2,
and proximity-induced superconductivity in III-V and group
IV semiconductor nanostructures, we complement our Collo-
quium by providing relevant reviews on these topics.
While we recognize that significant development is re-
quired before SOC-driven superconducting phenomena can
be applied in the field of spintronics or quantum technolo-
gies, sufficient progress has already been made both theoreti-
cally and experimentally where one can start to think about
potential areas of application. Using dissipationless super-
currents offers alternatives for energy-efficient information-
communication and quantum technologies. Just data cen-
ters alone are predicted to require 8% of globally generated
electrical power by 2030 (Jones, 2018). A potential solu-
tion may combine superconducting electronics with recent ad-
vances in spintronics (Hirohata et al., 2020; Tsymbal and Žu-
ti´
c, 2019) to seamlessly integrate logic and memory (Birge
and Houzet, 2019) and thereby overcome the von Neumann
bottleneck (Dery et al., 2012). More importantly, through
this review we hope to drive future innovations benefiting
fields like superconducting spintronics and Majorana physics
which will assist in solving material challenges that are key to
progress in these areas.
We start with a brief introduction to relevant theoretical and
experimental background of superconductivity in the presence
of SOC in hybrid structures, followed by recent developments
and, finally, concluding with open questions and highlight
promising research directions.
II. BACKGROUND
This section reviews basic concepts which build a basis for
the results outlined in the following sections. We start by de-
scribing SOC, specifically the Rashba and Dresselhaus mod-
els, in bulk materials and structures with inversion asymmetry.
We then introduce the physics emerging from SOC supercon-
ductivity in proximity structures and include a discussion on
theoretical methods that can be used to study such systems.
The purpose of this section is thus to provide the reader with
a set of theoretical concepts necessary to discuss the interest-
ing spintronics phenomena that arise due to the combination
of superconductivity and SOC in heterostructures.
A. Spin–orbit coupling
Coupling between the motion of an electron and its spin
stems from the fact that in the reference frame of the electron,
it is the positively charged lattice that moves. Moving charges
create a magnetic field, which may couple to the electron spin.
In a Lorentz-invariant formulation, a SOC term emerges, as
shown in the Dirac equation (Dirac, 1928)
mc2+V(r)i¯
hcσ·
i¯
hcσ·mc2+V(r)ψe
ψh=ε+mc2ψe
ψh,
(1)
and taking the nonrelativistic limit, ε,Vmc2, where ε
is the particle energy without its rest mass. Here, V(r)is
the lattice potential, mis the free electron mass, and σis
a vector of Pauli matrices. The resulting Hamiltonian is
H=p2/2m+V(r) + ¯
h/(4m2c2)σ·(V×p),for the elec-
tron wavefunction ψe, where irrelevant terms are discarded.
The last term represents SOC, large near a lattice site (Fabian
et al., 2007). Within second quantization, in the basis of the
Bloch functions, it takes the form (Samokhin, 2009),
HSO =
k
nn
ss
Qnn(k)·σssc
knsckns,(2)
where Qnnis a phenomenological model function which ex-
presses the coupling between momentum and spin, with nand
nband indices, and kthe crystal momentum. For a cen-
trosymmetric material, the terms Qnn vanish, SOC can only
be described by models containing at least two bands. How-
ever, in a noncentrosymmetric material a one-band model is
possible, nnQnnQin Eq. (2), while Q(k) = Q(k).
One can distinguish bulk and structure inversion asymmetry
(BIA, SIA), which lead to a spin splitting and SOC
HSO(k) = ¯
hσ·(k)/2,(3)
where (k)is the Larmor frequency for the electron spin
precession in the conduction band (Žuti´
cet al., 2004) or,
equivalently, SOC field. Here momentum scattering, (k)
is responsible for spin dephasing. Related SOC manifesta-
tions in semiconductors usually focuses on effective models
4
SIA
[111]
BIA
[001]
BIA
BIA [110]
110
110
001
100
010
FIG. 1: Vector fields (k)on a circular Fermi surface for
structure (SIA) and bulk (BIA) inversion asymmetry. Since
(k)is the spin quantization axis, the vector pattern is also
the pattern of the spin on the Fermi surface. As opposite
spins have different energies, the Fermi circle splits into two
concentric circles with opposite signs of spin; shown here
only for the SIA case, but the analogy extends to all
examples. The field for BIA [110] perpendicular to the plane,
with the magnitude varying along the Fermi surface. All
other cases have constant fields lying in the plane.
From Žuti´
cet al., 2004.
which capture the low-energy properties of the conduction
and valence bands. An example of BIA is the Dresselhaus
SOC (Dresselhaus, 1955), given by D= (2γ/¯
h)[kx(k2
y
k2
z),ky(k2
zk2
x),kz(k2
xk2
y)],where γis the SOC strength.
In two-dimensional (2D) systems with quantum confinement
along the unit vector ˆn,Dcan be linearized in k,
2D
Dk2
n[2nx(nykynzkz) + kx(n2
yn2
z)]ˆ
x+c.p., (4)
where k2
nis the expectation value of the square of the wave
number operator normal to the plane in the lowest subband
state while ˆn= (nx,ny,nz)is the confinement unit vector of
the quantum well, and c.p. denotes the cyclic index permuta-
tion. For a rectangular well of width a,k2
n= (π/a)2, while for
a triangular well k2
nis given in de Sousa and Das Sarma, 2003.
With a strong confinement, k2
k2
n, where kis the in-plane
(IP) wave vector (ˆn), cubic terms in kin Dfrom Eq. (4)
can be neglected.
For commonly considered quantum well confinements, one
obtains for [001]: 2D
Dk2
n(kx,ky,0), for [111]: 2D
D
k2
n(k×n), and for [110]: 2D
Dk2
nkx(1,1,0), as shown in
Fig. 1. Several features can be readily seen, BIA [100] dis-
plays a “breathing" pattern, while BIA [110] (k)is perpen-
dicular to the plane such that, within the linear in kapproxi-
mation, the perpendicular spins do not dephase.
An extensively studied SIA example is given by Bychkov-
Rashba (or just Rashba) SOC (Bychkov E. I. and Rashba,
1984), which arises in asymmetric quantum wells or in de-
formed bulk systems, expressed by
R=2α(k×n),(5)
where αparametrizes its strength and the inversion symmetry
is broken along the n-direction. We see in Fig. 1 that its func-
tional form, R, coincides with BIA 2D
Din [111] quantum
wells. A desirable property of Rashba SOC is that αis tunable
by an applied electric field. While these linearized forms of
the Rashba and Dresselhaus SOC are the most common mod-
els, there is an increasing interest in the study of phenomena
which go beyond their range of validity.
For example, in Rashba SOC there is a growing class of
materials where cubic terms in kcan play an important role,
or even be dominant (Alidoust et al., 2021). Finally, while
we have here focused on intrinsic SOC, we note that extrin-
sic SOC caused by impurities plays a key role in spintronics
both with and without superconductors, giving rise to impor-
tant contributions to spin Hall effects and spin relaxation (Žu-
ti´
cet al., 2004).
B. Validity of Rashba and Dresselhaus models
The validity of effective low-energy SIA and BIA SOC
models can be examined from electronic structure calcula-
tions, using first-principles, k·pmethod, or a tight-biding
model. Another contribution to Rashba-like spin splitting,
HL=p·E, arises in systems with localized orbital mo-
mentum, L(Park et al., 2012, 2011), where Eis the electric
field and the electric dipole moment, pL×k, is produced
by the asymmetric charge distribution. Rashba SOC strength
is renormalized by the orbital contribution, while local sym-
metry breaking can induce local orbital Rashba spin splitting
even in centrosymmetric systems (Lee and Kwon, 2020).
Going beyond Rashba and Dresselhaus model might be
necessary for interfacial SOC in junctions with interface-
induced symmetry reduction in the individual bulk con-
stituents and for multiorbital configurations (Mercaldo et al.,
2020). This is exemplified in an Fe/GaAs junction, where the
cubic and Tdsymmetries of bulk Fe and GaAs, respectively,
are reduced to C2v(Fabian et al., 2007; Žuti´
cet al., 2019).
Since the interfacial SOC is present only near the interface,
its effects can be controlled electrically via a gate voltage or
an applied external bias capable of pushing the carrier wave
function into or away from the interface. Interfacial SOC can
also be controlled magnetically, as it strongly depends on the
the orientation of Min the Fe layer, as illustrated from the
first-principles calculation in Figs. 2(b) and (c) (Gmitra et al.,
2013). The bias-dependence of the SOC can be inferred from
the transport anisotropy in Figs. 2(d) and (e).
While the resulting interfacial SOC for Fe/GaAs junction
corresponds neither to Rashba, nor Dresselhaus models, its
existence can be probed through tunneling anisotropic mag-
netoresistance (TAMR), which gives the dependence of the
tunneling current in a junction with only one magnetic elec-
trode on the orientation of M(Gould et al., 2004). For an IP
5
FIG. 2: (a) Schematic of a Fe/GaAs slab. For in-plane
TAMR, M, is rotated in the plane of Fe. (b) Angular k-space
dependence of the amplitude of the interfacial SOC field for
Malong the GaAs [1¯
10]direction (green arrow). (c) Same as
in (b) but for Malong the [110] direction (Gmitra et al.,
2013). The tunneling resistance R(φ)is normalized to its
φ=0 value, R[110]. Measurements for bias ±90 meV are
shown in (d) and (e), respectively (Moser et al., 2007). (f)
Angular dependence of the TAMR in the out-of-plane (OOP)
configuration. Left (right) panels correspond to CoPt/AlOx/Pt
(Co/AlOx/Pt) tunnel junctions. An extra Pt layer with strong
SOC yields in CoPt/AlOx/Pt two orders of magnitude larger
TAMR than in Co/AlOx/Pt. The insets show M
measurements in OOP magnetic fields (Park et al., 2008).
Adapted with permission from Žuti´
cet al., 2019.
rotation of Min Fig. 2(a), we can define TAMR as the nor-
malized resistance difference,
TAMR = (R(φ)R[110])/R[110],(6)
where R(φ=0)R[110]is the resistance along the [110] crys-
tallographic axis. The out-of-plane (OOP) TAMR is defined
analogously. TAMR appears because the electronic struc-
ture depends on the Morientation, due to SOC. The surface
or an interface electronic structure can strongly deviate from
its bulk counterparts and host pure or resonant bands. With
SOC, the dispersion of these states depends on the Morien-
tation (Chantis et al., 2007). As a result, the tunneling con-
ductance, which, in a crystalline junction, is very sensitive to
the transverse wave vector, develops both OOP and IP MR,
shown in Figs. 2(d)-(f), whose angular dependence reflects
the crystallographic symmetry of the interface. For example,
the TAMR inherits the C4vsymmetry for the Fe (001) sur-
face (Chantis et al., 2007) and the reduced C2vsymmetry for
the Fe(001)/GaAs interface (Moser et al., 2007).
Our prior discussion of SOC and its manifestations in the
normal-state properties have important superconducting coun-
terparts as well as enable entirely new phenomena, absent
in the normal state. Even when the SOC results in only a
small normal-state transport anisotropy, as shown in Figs. 2(d)
and (e), the superconducting analogs of such phenomena can
lead to much greater effects (Cai et al., 2021; Martínez et al.,
2020).
C. Triplet superconductivity
Conventional s-wave superconductors are well-described
by the Bardeen-Cooper-Schrieffer (BCS) microscopic theory.
The superconducting correlations consist of Cooper pairs in a
spin-singlet state and carry no net spin, unlike the proximity-
induced spin-triplet superconducting correlations. There are
materials believed to exhibit intrinsic triplet superconductivity
such as Bechgaard salts (Sengupta et al., 2001), UPt3(Joynt
and Taillefer, 2002), as well as the ferromagnetic supercon-
ductors (Aoki et al., 2011). A direct interaction between su-
perconductivity and SOC is also found in noncentrosymmetric
superconductors, where electron pairing is a mixure of spin-
singlet and spin-triplet (Smidman et al., 2017).
Through proximity effects, triplet superconducting correla-
tions can be generated using only conventional materials. In
S/F bilayers, the spin splitting in the latter leads to oscillations
in the pair correlation between the singlet and triplet spin con-
figurations due to a process akin to the Fulde-Ferrell-Larkin-
Ovchinnikov (FFLO) oscillations (Buzdin, 2005; Fulde and
Ferrell, 1964; Larkin and Ovchinnikov, 1965). Nevertheless,
such a coupling between S and homogeneous F is rapidly sup-
pressed as one moves away from the interface region, leading
to a short-range proximity effect. The situation is different in
F with an inhomogeneous Mdirection, where the spin of the
short-ranged triplet correlations is orthogonal to M. Here, the
short-ranged triplets decay over the coherence length of the
Cooper pairs in the F layer. If the orientation of Mchanges,
the triplet spin will obtain a component parallel to M. This
component, referred to as a long-ranged triplet component,
is not influenced by the spin splitting to the same degree as
their short-ranged counterparts. Remarkably, it may persist
for long distances as in nonmagnetic metals (Giroud et al.,
1998; Lawrence and Giordano, 1999; Petrashov et al., 1994,
1999), of the order pD/2πTin the diffusive limit, where D
is the diffusion coefficient of the F region and Tis the temper-
ature (Bergeret et al., 2001, 2005; Kadigrobov et al., 2001).
Engineering superconducting hybrid structures for generat-
ing spin-polarized triplets have been extensively studied. Us-
ing magnets with rare earth materials (holmium) with intrinsi-
cally inhomogeneous Min JJs, provides evidence of triplet
pair creation (Robinson et al., 2010; Sosnin et al., 2006).
摘要:

Colloquium:Spin-orbiteffectsinsuperconductinghybridstructuresMortenAmundsenNordita,KTHRoyalInstituteofTechnologyandStockholmUniversity,HannesAlfvénsväg12,SE-10691Stockholm,SwedenCenterforQuantumSpintronics,DepartmentofPhysics,NorwegianUniversityofScience&Technology,NO-7491Trondheim,Norway∗JacobLinde...

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