Disorder effects on the metastability of classical Heisenberg ferromagnets Moumita Naskar1Muktish Acharyya1Erol Vatansever2 3and Nikolaos G. Fytas3

2025-04-24 0 0 672.09KB 18 页 10玖币
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Disorder effects on the metastability of classical Heisenberg
ferromagnets
Moumita Naskar,1Muktish Acharyya,1, Erol Vatansever,2, 3 and Nikolaos G. Fytas3,
1Department of Physics, Presidency University,
86/1 College Street, Kolkata-700073, India
2Department of Physics, Dokuz Eylül University, TR-35160, Izmir, Turkey
3Centre for Fluid and Complex Systems,
Coventry University, Coventry, CV1 5FB, United Kingdom
(Dated: June 28, 2023)
Abstract
In the present work, we investigate the effects of disorder on the reversal time (τ) of classical
anisotropic Heisenberg ferromagnets in three dimensions by means of Monte Carlo simulations.
Starting from the pure system, our analysis suggests that τincreases with increasing anisotropy
strength. On the other hand, for the case of randomly distributed anisotropy, generated from
various statistical distributions, a set of results is obtained: (i) For both bimodal and uniform
distributions the variation of τwith the strength of anisotropy strongly depends on temperature.
(ii) At lower temperatures, the decrement in τwith increasing width of the distribution is more
prominent. (iii) For the case of normally distributed anisotropy, the variation of τwith the width
of the distribution is non-monotonic, featuring a minimum value that decays exponentially with
the temperature. Finally, we elaborate on the joint effect of longitudinal (hz) and transverse (hx)
fields on τ, which appear to obey a scaling behavior of the form τhn
zf(hx).
Electronic address: muktish.physics@presiuniv.ac.in
Electronic address: nikolaos.fytas@coventry.ac.uk
1
arXiv:2210.05510v2 [cond-mat.stat-mech] 27 Jun 2023
I. INTRODUCTION
The metastable behavior of a ferromagnet is an interesting field of modern research with
important technological applications [1, 2]. It is well-known today that the so-called switch-
ing time (or reversal time τ), a critical parameter of this process, plays a key role in the speed
of recording in magnetic storage devices [3]. The whole problem of metastability dates back
to 1935, where the classical theory of nucleation was developed by Becker and Döring [4],
predicting the growth of supercritical droplets. These predictions of the different regimes
of such growth depending on the magnitude of the applied magnetic field were successfully
verified by extensive Monte Carlo simulations in Ising [5] and Blume-Capel ferromagnets [6],
as well as in generalized spin-sanisotropic models [7].
Over the years, most numerical approaches of reversal phenomena dealing with the growth
of supercritical clusters, the decay of metastable volume fraction, and their dependencies
on the applied field and temperature, focused on pure ferromagnetic systems of discrete
symmetric Ising and Blume-Capel models. A straightforward extension would be then to
consider the case of continuous symmetric spin models, such as the classical Heisenberg
model. Indeed, a few papers have already shed some light in this context: The magneti-
zation switching in the classical anisotropic Heisenberg ferromagnet was studied by Monte
Carlo simulations and the dynamics of coherent spin rotation was detected in the limit of
low anisotropy [8]. Later on, the reversal properties were studied in classical anisotropic
ferromagnetic and antiferromagnetic bilayer Heisenberg models and it was observed that
the magnetization behavior is different at each branch of the hysteresis loop as well as
the exchange-bias behavior [9]. More recently, the problem was investigated in the anti-
ferromagnetic anisotropic Heisenberg chain [10] and in a Van-der-Waals magnet where a
strain-sensitive magnetization reversal was reported [11]. This latter work indicated that
lattice deformation plays a major role in the reversal process, as it may lead to random
variations of the crystal field (anisotropy) acting on the spins of the system.
In all aforementioned studies regarding the anisotropic classical Heisenberg ferromagnet,
uniform anisotropy was used for simplicity. At this point several intriguing questions may
be raised: (i) What will be the effect of a random anisotropy on the reversal phenomena in
the classical Heisenberg ferromagnet? (ii) How does the nature of the statistical distribution
of the anisotropy affect the reversal of magnetization and other properties of the system? To
2
the best of our knowledge, all these open fundamental aspects have not yet been addressed so
our understanding of metastable phenomena in a random environment is rather limited – see
Refs. [12, 13] for some particular exceptions. In the present work, we make one step forward
in this direction by studying via Monte Carlo simulations the three-dimensional anisotropic
classical Heisenberg ferromagnet with the disorder, generated by a set of random anisotropy
distributions.
The rest of the paper is organized as follows: Section II provides a description of the
model together with an outline of the simulation scheme. The numerical results and scaling
analysis are reported in Sec. III. This paper concludes with a summary and outlook in
Sec. IV.
II. MODEL AND NUMERICS
The classical anisotropic (uniaxial and single-site) Heisenberg model with nearest-
neighbor ferromagnetic interactions in the presence of an external magnetic field is described
by the following Hamiltonian
H=JX
ij
Si·SjX
i
Di(Sz
i)2hX
i
Si,(1)
where Si(Sx
i, Sy
i, Sz
i)represents a classical spin vector with |S|= 1 (or (Sx
i)2+(Sy
i)2+(Sz
i)2=
1) which is allowed to take any (unrestricted) angular orientation in the vector space. The
first term in the Hamiltonian corresponds to nearest-neighbor (ij) ferromagnetic (J > 0)
spin-spin interaction. The parameter Diappearing in the second term denotes the strength
of uniaxial anisotropy favoring the z-axis alignment of the spin vector. Note that the limit
D→ ∞ corresponds to the Ising ferromagnet, whereas for D= 0 Eq. (1) reduces to the
isotropic Heisenberg Hamiltonian. Finally, the last term in the Hamiltonian (1) stands for the
interaction of individual spins with the externally applied magnetic field vector h(hx, hy, hz).
The reversal of magnetization is studied mainly in the presence of a longitudinal field hz
unless otherwise stated. However, in the last part of our study, we also present the influence
of an additional transverse field (hx) on the reversal mechanism, along with the longitudinal
field.
We used Monte Carlo simulations of Metropolis type to study the model of Eq. (1)
on simple cubic lattices with periodic boundary conditions and linear dimension L, where
3
typically L= 50 (more information on the numerical details is given in Appendix A). In
all our numerical experiments, L3such spin updates define one Monte Carlo step per site,
which also sets the time unit of our simulations. We also fix J=kB= 1 to properly set the
temperature scale.
Finally some comments about errors and fitting analysis: Unless otherwise stated, we
always perform the necessary statistical averaging to increase the accuracy of our data
(more details are given explicitly in the plots of Sec. III) and compute standard errors [15].
For the fits, we implement the χ2test of goodness of fit [16]. Specifically, the Qvalue of
our χ2test is the probability of finding a χ2value that is even larger than the one actually
found from our data. We consider a fit as being fair only if 10% <Q<90%.
III. RESULTS AND DISCUSSION
The first port of call in our study is to secure a rough estimate for the critical temper-
ature of the Heisenberg model so that we assure that the system lies well below its critical
temperature. Although in previous works [17] we observed no such detectable discontinuity
in the behavior of the metastable lifetime across the phase boundary of the ferromagnetic-
paramagnetic transition, still, in the present study, we follow the standard way of studying
the reversal time or the metastable lifetime below the critical temperature. As the pre-
cise determination of the critical temperature is definitely not necessary here, we follow the
simplest practice for locating an approximate estimation of the critical temperature. The
method refers to the detection of the pseudo-critical temperature, T
L, at which the magnetic
susceptibility χobtained via
χ=Nβm2⟩−⟨m2(2)
attains a peak for a relatively large system size L. In the above Eq. (2), N=L3,β= 1/T ,
and m=pm2
x+m2
y+m2
zdenotes the magnetization of the system, where mx= (PiSx
i)/N,
my= (PiSy
i)/N, and mz= (PiSz
i)/N. Figure 1(a) presents the T-variation of χfor a
system with linear size L= 20 and for various values of Dand Fig. 1(b) clearly illustrates
that the pseudo-critical temperatures obtained increase with increasing uniform anisotropy
D. Note that the temperature is varied in steps of δT = 102so that the maximum error
in the T
L-determination is δT
L2.102.
The metastable lifetime (or reversal time) τ, the crucial parameter of our analysis, is
4
摘要:

DisordereffectsonthemetastabilityofclassicalHeisenbergferromagnetsMoumitaNaskar,1MuktishAcharyya,1,∗ErolVatansever,2,3andNikolaosG.Fytas3,†1DepartmentofPhysics,PresidencyUniversity,86/1CollegeStreet,Kolkata-700073,India2DepartmentofPhysics,DokuzEylülUniversity,TR-35160,Izmir,Turkey3CentreforFluidand...

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