Persistent motion of a Brownian particle subject to repulsive feedback with time delay Robin A. Koppand Sabine H. L. Klapp Institut f ur Theoretische Physik

2025-05-02 0 0 1.86MB 16 页 10玖币
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Persistent motion of a Brownian particle subject to repulsive feedback with time delay
Robin A. Koppand Sabine H. L. Klapp
Institut f¨ur Theoretische Physik,
Technische Universit¨at Berlin,
Hardenbergstr. 36, D-10623 Berlin, Germany
(Dated: March 7, 2025)
Based on analytical and numerical calculations we study the dynamics of an overdamped colloidal
particle moving in two dimensions under time-delayed, non-linear feedback control. Specifically, the
particle is subject to a force derived from a repulsive Gaussian potential depending on the difference
between its instantaneous position, r(t), and its earlier position r(tτ), where τis the delay
time. Considering first the deterministic case, we provide analytical results for both, the case
of small displacements and the dynamics at long times. In particular, at appropriate values of the
feedback parameters, the particle approaches a steady state with a constant, non-zero velocity whose
direction is constant as well. In the presence of noise, the direction of motion becomes randomized
at long times, but the (numerically obtained) velocity autocorrelation still reveals some persistence
of motion. Moreover, the mean-squared displacement (MSD) reveals a mixed regime at intermediate
times with contributions of both, ballistic motion and diffusive translational motion, allowing us to
extract an estimate for the effective propulsion velocity in presence of noise. We then analyze the
data in terms of exact, known results for the MSD of active Brownian particles. The comparison
indeed indicates a strong similarity between the dynamics of the particle under repulsive delayed
feedback and active motion. This relation carries over to the behavior of the long-time diffusion
coefficient Deff which, similarly to active motion, is strongly enhanced compared to the free case.
Finally we show that, for small delays, Deff can be estimated analytically.
I. INTRODUCTION
Within the last years, feedback (closed-loop) control
of colloidal systems, that is, nano- to micron-sized parti-
cles in a thermally fluctuating bath of solvent particles,
has become a focus of growing interest. Conceptually,
feedback control implies that the dynamics of a system
is subject to a protocol depending on an internal vari-
able, i.e., internal information from the system. This
concept is already widely used in other fields of physics
(and related sciences) and on many different length- and
time scales [1, 2], examples ranging from the stabiliza-
tion of exotic quantum states and quantum computation
over control of transport of (passive) colloids to switching
processes in neurosystems, applications in robotics and
cars, and chaos control of satellites. In contrast, the use
and design of feedback control in colloidal or, more gen-
erally, soft matter systems is a rather new development.
Recent experimental applications include control of DNA
molecules by feedback-driven temperature fields [3, 4] or
optical traps [5], magnetic feedback control of cells [6],
electrophoretic feedback control of nanoparticles [7], col-
loids in a electrokinetic feedback trap [8], in optical line
traps [9], and feedback cooling of nanoparticles [10].
A new, exciting field of application is feedback con-
trol of active (self-propelled) colloids which move au-
tonomously due to an intrinsic source of energy. Con-
trol of the translational or rotational motion of active
r.kopp@tu-berlin.de
sabine.klapp@tu-berlin.de
colloids can be realized, e.g., by photon nudging and by
adaptive light fields [11–20]. Interest in this topic is trig-
gered by the immense body of work on active particles
showing intriguing collective behaviors such as swarming
and clustering. Feedback control of such systems offers
a way of modelling living matter involving not only au-
tonomous motion, but also communication, sensing and
thereby new types of self-organization. In addition to
these efforts, feedback control of colloids is interesting, on
a fundamental level, to study its interplay with thermo-
dynamics and information exchange in small stochastic
systems [8, 21–25] on the basis of stochastic thermody-
namics [26].
In any realistic setup of feedback control (and simi-
larly in biological systems), there is some time lag (or
time delay) between the reception of information (e.g.,
via a camera) and the actual control. Similarly, biological
living systems with feedback mechanisms often exhibit
some degree of sensorial delay [17], communication delay
[27], or, more generally, memory effects due to viscoelas-
tic environments [28]. Thus, the idea of instantaneous
feedback is often an idealization. Moreover, there is now
increasing awareness that this time delay is not per se an
annoyance, but can rather be an important ingredient to
observe and stabilize certain dynamical behavior. The
constructive role of time delay has already been shown in
other contexts [1, 2, 29] including chaos control [30, 31],
[32], laser systems [33, 34], chemical oscillatory systems
[35] and reaction networks [36]. Recently is has been
shown that time delay has also important consequences
for the thermodynamics of feedback-controlled systems
[24, 37, 38].
In colloidal systems, time-delayed feedback has already
arXiv:2210.03182v3 [cond-mat.soft] 6 Mar 2025
2
been shown to create intriguing effects. Examples in the
field of transport of (one-dimensional) passive colloidal
systems include current reversals [39] and enhancements
[9, 40, 41] in ratchet and tilted washboard systems, but
also band formation in two-dimensional interacting col-
loidal systems with collective time-delayed feedback [42].
Moreover, recent studies of (time-delayed) feedback con-
trol in active systems [13–15] have revealed new effects
such as delay-induced clustering and swarming [17, 43–
45]. Despite the increasing awareness of the relevance of
delay and feedback effects in colloidal systems, theoreti-
cal studies of specific model systems are still rare. This
is mainly due to the non-Markovianity of the underlying
stochastic equations of motion, making explicit calcula-
tions challenging. Indeed, exact results only exist for lin-
ear models [46–49]. However, in real colloidal systems,
the interactions and forces involved are typically nonlin-
ear. Motivated by these developments, we here present
a theoretical study of a particular nonlinear model of a
colloidal particle under time-delayed feedback. Specifi-
cally, we consider the two-dimensional translational mo-
tion of a single, spherical colloid subject to a repulsive
force generated by a Gaussian potential centered around
the particle position at an earlier time tτ. Thus, the
position acts as a stochastic variable on which the control
is performed. Our model differs in several aspects from
earlier ones (see, e.g. [40, 41]). We here consider repul-
sive feedback, rather than the often studied case of trap-
ping a particle by an attractive potential (stemming, e.g.,
from an optical tweezer). We note that similar nudging
mechanisms have already been used in the context of the
“photo-nudging” method for Janus particles [11–15, 50].
A second difference is that the force is nonlinear in the
particle position and finite in range. Thus, although our
model is not directly designed to describe a specific ex-
periment and is, in this sense, hypothetical, it allows us
to focus exclusively on several important features of a
control scheme for Brownian particles: time-delay, repul-
sion, and nonlinearity.
Explicit results are obtained based on analytical con-
siderations in some limiting cases, as well as on numer-
ical solution of the corresponding (overdamped) non-
Markovian Langevin equation. The first main result of
our study is that for appropriate values of delay time and
strength of repulsion, and in the absence of noise, the par-
ticle develops a stationary state characterized by a con-
stant velocity vector. Second, thermal fluctuations lead
to a randomization of the direction of motion, but the
particle still possesses a persistence of motion and a con-
stant magnitude of speed (after noise-averaging). This
is reminiscent of the stochastic behavior of self-propelled
particles, and indeed we identify close similarities. In
particular, we discuss relations to the prominent model
of active Brownian particles (ABP) [51]. For this model,
which is widely used also to explain experimental data
(see, e.g. [52, 53]), there exists a closed analytical expres-
sion for the mean-squared displacement which we utilize
to fit and interpret our numerical data. Further, the ABP
model is one of the best studied systems concerning the
collective behavior induced by activity [53, 54]. Thus, es-
tablishing a link to the ABP model will provide us with
a basis for future investigation of the collective behavior
of our model. By investigating, in the present study, the
single-particle relations between the different models we
make a first step to establishing a link between feed-back
controlled and active matter.
The rest of the paper is organized as follows: In the
following section II we introduce our model and the cor-
responding overdamped Langevin equation governing the
dynamics of the system. Subsequently we study, first, the
deterministic limit in Sec. III, using a combination of
analytical and numerical methods. We then present our
results for the full, nonlinear stochastic system, based on
Brownian dynamics simulations, in Sec. IV. Our conclu-
sions are summarized in Sec. V.
II. MODEL
We consider the two-dimensional motion of a Brow-
nian particle in the x-yplane. In addition to thermal
fluctuations due to a coupled heat bath at temperature
T, the particle is subject to a time-delayed feedback
force Fdepending on both, its instantaneous position
r(t)=(x(t), y(t))Tand its position at an earlier time,
r(tτ), where τis the (discrete) delay time. The parti-
cle’s motion at times t > 0 is governed by the overdamped
Langevin equation
γdr
dt =F(r(t),r(tτ)) + ξ(t),(1)
where γis the friction coefficient, and the position at ear-
lier times t[τ, 0] is determined by the history func-
tion Φ(t). Furthermore, ξrepresents a two-dimensional,
Gaussian white noise with zero mean and correlation
function ξα(t)ξβ(t)= 2γkBT δαβδ(tt) where α,β
are the cartesian components of the noise vector ξ, and
kBT(with kBbeing the Boltzmann constant) is the ther-
mal energy. The diffusion constant of the free particle
motion (F=0) follows from the Stokes-Einstein relation
D=kBT.
Within our model, the feedback force Fis derived from
a Gaussian feedback potential involving the displacement
r(t)r(tτ), that is,
V(r(t),r(tτ)) = Aexp (r(t)r(tτ))2
2b2!,(2)
yielding
F=−∇rV(r(t),r(tτ))
=A
b2(r(t)r(tτ)) exp (r(t)r(tτ))2
2b2!.(3)
We choose the feedback strength A > 0, representing re-
pulsive feedback whose range is determined by the width
3
F
r(tτ)
r(t)
V(r(t),r(tτ))
FIG. 1. Schematic of the repulsive Gaussian delayed feedback
potential V. At each time t, the Gaussian is centered around
the earlier position r(tτ), resulting in a “pushing” force (red
arrow) directed along the difference vector r(t)r(tτ).
of the Gaussian, b(b > 0). The width of the feed-
back potential serves as the length scale in our system.
An illustration of the “bump”-like potential is given in
Fig. 1. Physically, the potential (2) can be interpreted
as a source of a “nudge” following the particle with some
delay. Such a potential could, in principle, be created
by optical forces [15, 19, 50, 55–57]. We note that, dif-
ferent to the often used harmonic potentials leading to
linear feedback forces [58], the potential (2) and the force
(3) decay to zero when the displacement within one de-
lay time, r(t)r(tτ), increases to large values. The
finite range is indeed advantageous when using Eq. (2)
in a many-particle system with periodic boundary con-
ditions. We also note, from the perspective of control
theory, the feedback force has “Pyragas” form [30, 31]
since it only depends on the difference between r(t) and
r(tτ). Thus, the force vanishes trivially if τ= 0; in
this case, our model reduces to that of a free Brownian
particle. Note, however, that the feedback force also van-
ishes when the particle is at rest, that is, r(tτ) = r(t),
or when it moves in a cyclic fashion with period τ.
Inserting the expression for the force (3) into Eq. (1),
the complete equation of motion reads
γdr
dt =A
b2(r(t)r(tτ)) exp (r(t)r(tτ))2
2b2!
+ξ(t).(4)
Due to the presence of time delay, the particle’s dynam-
ics defined by Eq. (4) is strongly non-Markovian (where
“strongly” refers to the fact that the kernel emerging
when we write the right side as a convolution over past
times is a delta peak located at a finite time τ[59]). As a
consequence, several tools well established for Markovian
Brownian systems (such as the link between Langevin
and Fokker Planck descriptions) do not straightforwardly
apply. More mathematically spoken, Eq. (4) represents
a stochastic delay differential equation (SDDE) which is,
furthermore, non-linear due to the Gaussian shape of the
underlying potential. Even in the absence of noise, the
resulting differential equation (DDE) formally becomes
infinite-dimensional due to the presence of the continuous
history function Φ(t). In recent years, a number of re-
sults have been obtained for deterministic DDEs [60–62],
as well as for linear SDDEs see, e.g., [46–49]. However,
here we are dealing with a nonlinear SDDE for which, to
our knowledge, no full analytical solution exists. Still, we
can analytically consider some limiting cases, which we
will discuss in the subsequent Sections III and IV. In ad-
dition, we study the particle dynamics given by Eq. (4)
and its deterministic limit numerically using Brownian
Dynamics (BD) simulations. Some technical details of
the numerical calculations are given in Appendix A.
III. DETERMINISTIC LIMIT
We start by considering the deterministic limit of
Eq. (4) defined by ξ=0, which may be realized by
setting the temperature Tto zero. In this way we can
explore the role of delay alone, thereby providing a use-
ful starting point for the later investigation of the noisy
case.
A. Linear behavior
Some first insights can already be obtained by investi-
gating the behavior at small displacements |r(t)r(t
τ)| ≪ 2b. In this case, we can expand the force (3)
up to first order in the displacement, yielding the linear
equation
γ˙
r=A
b2(r(t)r(tτ)) .(5)
In deriving Eq. (5) we have used that the Hessian ma-
trix H(r) with elements Hαβ (r) = 2V /∂xαxβ(with
V(r) being the feedback potential) is diagonal at r= 0,
and Hαα(0) = A/b2. As a consequence of the diago-
nality, each component xαof rcan be considered sepa-
rately. The resulting scalar, linear DDEs are indeed well
studied. For example, it is well known [63–65] that the
(fixed) point r=r0with xα=const is marginally stable
in the sense that a perturbation exp[µt] (with µbe-
ing a complex number) remains constant, that is, µ= 0.
Physically, this expresses the metastability of a particle
on a “parabolic mountain” [58]. Moreover, explicit solu-
tions of the linear equation (5) can be constructed in a
piecewise manner by using the method of steps [60, 61].
For a given history function Φ(t) with components Φα(t)
4
(defined in the interval t[τ, 0]), the solution in the
first interval t[0, τ] follows as
xα= exp At
γb2α(0)
A
γb2Zt
0
dtexp A(t)
γb2Φα(tτ)(6)
which shows directly the dependency on the history. In
particular, if the particle was at rest at some fixed po-
sition (Φ=r0), it stays where it is (as expected from
the marginal stability) for all values of the prefactor
A/b2. This then also holds for the later time intervals
[, (n+ 1)τ] (with n= 1,2, . . .). A more interesting
situation for the present study occurs if the particle had
moved with a constant velocity v0, that is, Φ=v0t,
t[τ, 0]. The corresponding explicit solution for t > 0
up to time 2τis given in the Appendix B. It turns out
that the behavior of xα(t) (and the corresponding veloc-
ity) crucially depends on the value of the dimensionless
parameter b2. If this parameter is smaller than one,
the particle just approaches a constant position and the
velocity dies off to zero. In contrast, if b2>1,
the position and the corresponding velocity continue to
increase unboundly. Finally, at the “threshold” value
b2= 1, the behavior just remains identical to that
given by the history, that is, the particle continues to
move with the velocity v0. An illustration of these be-
haviors is given in Fig. 2 (dashed lines), where the history
is characterized by a one-dimensional velocity (generat-
ing one-dimensional motion), v0=v0ˆ
x,t[τ, 0].
B. Nonlinear behavior and steady state
We now consider the full, nonlinear (deterministic) sys-
tem. The corresponding DDE (4) with ξ=0cannot
be solved any more by the method of steps, such that
we utilize a numerical solution to obtain the full trajec-
tory r(t) in dependence of the history Φ(t). Examples
are shown in Fig. 2 (solid lines) where we focus (again)
on an initial velocity along the x-axis. At small times
t/τ > 0, the solution agrees with that obtained for the
(linear) case describing small displacements, as it should
do. The further time dependence of the nonlinear system
again crucially depends on the dimensionless parameter
b2. In particular, for b21 the nonlinear sys-
tem comes to rest in the sense that the position settles
and the velocity vanishes. Note that this is consistent
with the linear case for b2<1, but not for the
“threshold” value b2= 1, where the linear system
is fully governed by the history. Moreover, a crucial dif-
ference between the systems emerges when b2>1.
Here, the nonlinear system governed by the full, Gaussian
feedback develops a stationary state characterized by a
constant velocity v. This velocity can be determined
analytically as follows.
Let us assume that such a state develops. We then
have ˙
r=vand r(t)r(tτ) = vτ. Inserting this
1 0 1 2
t/τ
0.5
0.0
0.5
1.0
1.5
2.0
2.5
3.0
3.5
x(t)/b
(a)
nonlinear linear
b2= 0.25
b2= 1.0
b2= 1.75
b2= 4.0
b2= 0.25
b2= 1.0
b2= 1.75
b2= 4.0
02468
t/τ
0
1
2
3
4
˙x(t)τ /b
vτ/b
vτ/b
(b)
nonlinear linear
b2= 0.25
b2= 1.0
b2= 1.75
b2= 4.0
b2= 0.25
b2= 1.0
b2= 1.75
b2= 4.0
FIG. 2. Numerical results for the time dependence of the
position (a) and velocity (b) of the particle subject to nonlin-
ear, Gaussian feedback in the deterministic limit (for a his-
tory with constant (one-dimensional) velocity v0=v0ˆ
x, i.e.,
Φ=v0t). Included are the analytical results for the linearized
case (small displacements [see Eq. (5)]). The curves are la-
belled according to the value of the dimensionless parameter
b2.
into the deterministic version of Eq. (4) we obtain an
implicit equation for the long-time velocity,
v=
γb2vexp (vτ)2
2b2!,(7)
yielding
|v|=±2b
τsln γb2
.(8)
摘要:

PersistentmotionofaBrownianparticlesubjecttorepulsivefeedbackwithtimedelayRobinA.Kopp∗andSabineH.L.Klapp†Institutf¨urTheoretischePhysik,TechnischeUniversit¨atBerlin,Hardenbergstr.36,D-10623Berlin,Germany(Dated:March7,2025)Basedonanalyticalandnumericalcalculationswestudythedynamicsofanoverdampedcollo...

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